I assume you mean vignette in which case just checked in Picasa where you can choose any colour under the sun. I still use Picasa as part of my final stage in my workflow on a photograph, even though I have PE10, CS4 & LR4.
Just checked in LR and can't see how to add a colour vignette unless I am missing a point
open your image
ctrl+j
use the picker to chose any colour you want
alt+backspace
use the rectangular or oval marque tool to cut out the area you don't want to vignette
select feather > 170
hit backspace
then change the opacity to what you want.
My method in a new layer, set the colour I want as background colour (on the colour picker) then radial gradient, drag from the center out and set the layer blend mode to mulitply, ajust opacity to suit.
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