You can copy the contents that way, but it won't be a copy of the disk if it's bootable. You'll need to use special software to do that and there are lots to choose from.
Macrium is pretty good for Windows work, Carbon Copy Cloner is good for Macs. If you're happy on the command line, rsync will work on any Unix/Linux machine (including the versions on both Apple and later versions of Windows).
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