I personnaly prefere silver effects pro (for photoshop) but theres tons of free actions etc which do a decent job, to be fair CS5 does a good job on it's own.
Don't use desaturate, it's about the worst method.
What software are you using?
Usually I prefer to use RAW images saved to TIFF 24-bit and split to RGB channels. I can dump the channels into layers and set different opacity levels and paint in and out what gives the best result before combining (flatening) the image.
In this process JPEG images may look blotched here and there due to compression and in-camera colour interpolation.
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